Publications: Annotated

Imaging nanoscale Fermi-surface variations in an inhomogeneous superconductor

W. D. Wise, Kamalesh Chatterjee, M. C. Boyer, Takeshi Kondo, T. Takeuchi, H. Ikuta, Zhijun Xu, Jinsheng Wen, G. D. Gu, Yayu Wang, E. W. Hudson

Nature Physics, Volume 5, Issue 3, pp. 213-216 (2009) [Preprint PDF]

Particle–wave duality suggests we think of electrons as waves stretched across a sample, with wavevector k proportional to their momentum. Their arrangement in 'k-space', and in particular the shape of the Fermi surface, where the highest-energy electrons of the system reside, determine many material properties. Here we use a novel extension of Fourier-transform scanning tunnelling microscopy to probe the Fermi surface of the strongly inhomogeneous Bi-based cuprate superconductors. Surprisingly, we find that, rather than being globally defined, the Fermi surface changes on nanometre length scales. Just as shifting tide lines expose variations of water height, changing Fermi surfaces indicate strong local doping variations. This discovery, unprecedented in any material, paves the way for an understanding of other inhomogeneous characteristics of the cuprates, such as the pseudogap magnitude, and highlights a new approach to the study of nanoscale inhomogeneity in general.

Scanning tunneling microscopy of the 32 K superconductor (Sr1-xKx)Fe2As2

M. C. Boyer, Kamalesh Chatterjee, W. D. Wise, G. F. Chen, J. L. Luo, N. L. Wang, E. W. Hudson

eprint arXiv:0806.4400 [Preprint PDF]

The discovery of high temperature superconductivity in La[O1-xFx]FeAs at the beginning of this year has generated much excitement and has led to the rapid discovery of similar compounds with as high as 55 K transition temperatures. The high superconducting transition temperatures are seemingly incompatible with the electron-phonon driven pairing of conventional superconductors, resulting in wide speculation as to the mechanism and nature of the superconductivity in these materials. Here we report results of the first scanning tunneling microscopy study of the 32 K superconductor (Sr1-xKx)Fe2As2. We find two distinct topographic regions on the sample, one with no apparent atomic corrugation, and another marked by a stripe-like modulation at double the atomic periodicity. In the latter the stripes appear to modulate the local density of states, occasionally revealing a Δ = 10 mV gap with a shape consistent with unconventional (non-s wave) superconductivity.

Charge-density-wave origin of cuprate checkerboard visualized by scanning tunnelling microscopy

W. D. Wise, M. C. Boyer, Kamalesh Chatterjee, Takeshi Kondo, T. Takeuchi, H. Ikuta, Yayu Wang, E. W. Hudson

Nature Physics, Volume 4, Issue 9, pp. 696-699 (2008) [Preprint PDF]

One of the main challenges in understanding high-Tc superconductivity is to disentangle the rich variety of states of matter that may coexist, cooperate or compete with d-wave superconductivity. At centre stage is the pseudogap phase, which occupies a large portion of the cuprate phase diagram surrounding the superconducting dome. Using scanning tunnelling microscopy, we find that a static, non-dispersive, 'checkerboard'-like electronic modulation exists in a broad regime of the cuprate phase diagram and exhibits strong doping dependence. The continuous increase of checkerboard periodicity with hole density strongly suggests that the checkerboard originates from charge-density-wave formation in the antinodal region of the cuprate Fermi surface. These results reveal a coherent picture for static electronic orderings in the cuprates and shed important new light on the nature of the pseudogap phase.

Visualization of the interplay between high-temperature superconductivity, the pseudogap and impurity resonances

Kamalesh Chatterjee, M. C. Boyer, W. D. Wise, Takeshi Kondo, T. Takeuchi, H. Ikuta, E. W. Hudson

Nature Physics, Volume 4, Issue 2, pp. 108-111 (2008).

Introduction (News & Views): Superconductivity: Bring on the real resonance (W.-S. Lee & Z.-X. Shen)

In conventional superconductors, the superconducting gap in the electronic excitation spectrum prevents scattering of low-energy electrons. In high-temperature superconductors (HTSs), an extra gap, the pseudogap, develops well above the superconducting transition temperature TC. Here, we present a new avenue of investigating the pseudogap state, using scanning tunnelling microscopy (STM) of resonances generated by single-atom scatterers. Previous studies on the superconducting state of HTSs have led to a fairly consistent picture in which potential scatterers, such as Zn, strongly suppress superconductivity in an atomic-scale region, while generating low-energy excitations with a spatial distribution—as imaged by STM—indicative of the d-wave nature of the superconducting gap. Surprisingly, we find that similar native impurity resonances coexist spatially with the superconducting gap at low temperatures and survive virtually unchanged on warming through TC. These findings demonstrate that properties of impurity resonances in HTSs are not determined by the nature of the superconducting state, as previously suggested, but instead provide new insights into the pseudogap state.

Imaging the two gaps of the high-temperature superconductor Bi2Sr2CuO6+x

M. C. Boyer, W. D. Wise, Kamalesh Chatterjee, Ming Yi, Takeshi Kondo, T. Takeuchi, H. Ikuta, E. W. Hudson

Nature Physics, Volume 3, Issue 11, pp. 802-806 (2007) [Preprint PDF]

The nature and behaviour of electronic states in high-temperature superconductors are the centre of much debate. The pseudogap state, observed above the superconducting transition temperature, TC, is seen by some as a precursor to the superconducting state. Others view it as a competing phase. Recently, this discussion has focused on the number of energy gaps in the system. Some experiments indicate a single energy gap, implying that the pseudogap is a precursor state. Others indicate two, suggesting that it is a competing or coexisting phase. Here, we use temperature-dependent scanning tunnelling spectroscopy of (Bi1-yPby)2Sr2CuO6+x to clarify the situation. We find a previously unobserved narrow and homogeneous gap that vanishes near TC, superimposed on the typically observed inhomogeneous and broad gap, which is only weakly temperature dependent. These results not only support the two-gap picture, but also explain previously troubling differences between scanning tunnelling microscopy and other experimental measurements.